Title should be changed to reindeer, not deer. As those are domesticated by the Sami people. Then it makes more sense and should not be a major task, since they are regularly caught to be ear-marked for example. In general a good idea IMO.
For deer it would be trickier, but I imagine you could somehow do it by setting up feeding stations (pretty common with hunters) and spray them when they approach it. But it would be messy. Now my imagination is wandering, please stop me.
Wouldn’t that be a death sentence by making them super easy for predators to spot?
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It's not possible at all to do this for white-tailed deer. The does and fawns don't grow antlers. My state, NJ, has a population of over 100,000 deer and average densities over 100 individuals per square mile (with some areas over double that).